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Adv Mater 10:901 915 Qi B, Tong X, Zhao Y, Zhao Y 2008 A micellar route to layer by layer assembly of hydrophobic functional polymers Macromolecules 41:3562 3570 Qin S, Geng Y, Discher DE, Yang S 2006 Temperature controlled assembly and release from polymer vesicles of poly(ethylene oxide) block poly(N isopropylacrylamide) Adv Mater 18:2905 2909 Rapoport N, Pitt WG, Sun H, Nelson JL 2003 Drug delivery in polymeric micelles: from in vitro to in vivo J Control Release 91:85 95 Ravi P, Sin SL, Gan LH, Gan YY, Tam KC, Xia XL, Hu X 2005 New water soluble azobenzene containing diblock copolymers: synthesis and aggregation behavior Polymer 46:137 146 Sakai H, Matsumura A, Yokoyama S, Saji T, Abe M 1999 Photochemical switching of vesicle formation using an azobenzene modi ed surfactant J Phys Chem B 103:10737 10740.

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(V)' 0.389 0.358 0.354 0.348 0.337 0.328 0.252 0.206 0.161 0.035 -0.251 -0.372 -0.316 -0.295 -0.253 -0.195 0.048 0.372 0.182 -0.225 -0.364 -0.481 -0.408 -0.273 -0.069

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Schilli CM, Zhang M, Rizzardo E, Thang SH, Chong YK, Edward K, Karlsson G, Muller AHE 2004 A new double responsive block copolymer synthesized via RAFT poly merization: poly(N isopropylacrylamide) block poly(acrylic acid) Macromolecules 37:7861 7866 Shang TG, Smith KA, Hatton TA 2003 Photoresponsive surfactants exhibiting unusually large, reversible surface tension changes under varying illumination conditions Lang muir 19:10764 10773 Shin JY, Abbott NL 1999 Using light to control dynamic surface tensions of aqueous solutions of water soluble surfactants Langmuir 15:4404 4410 Shinkai S, Matsuo K, Harada A, Manabe O 1982 Photocontrol of micellar catalyses J Chem Soc Perkin Trans 2:1261 1265 Simmons JM, In I, Campbell VE, Mark TJ, Leonard F, Gopalan P, Eriksson MA 2007 Optically modulated conduction in chromophore functionalized single wall carbon nanotubes Phys Rev Lett 98:086802(1 4) Sin SL, Gan LH, Hu X, Tam KC, Gan YY 2005.

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Photochemical and thermal isomeriza tion of azobenzene containing amphiphilic diblock copolymers in aqueous micellar aggregates and in lm Macromolecules 38:3943 3948..

-38.4 -34.5 -68.3 -67.2 -32.5 -63.3 -24.3 -19.9 -15.5 -3.4 24.2 35.9 -30.5 -28.5 -24.4 -18.8 4.6 35.9 -17.6 21.8 35.1 -46.4 -39.3 -26.4 -6.7

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Su W, Zhao H, Wang Z, Li Y, Zhang Q 2007 Sphere to disk transformation of micro particle composed of azobenzene containing amphiphilic diblock copolymers under irradiation at 436 nm Eur Polym J 43:657 662 Taillefer J, Jones MC, Brasseur N, Van Lier JE, Leroux JC 2000 Preparation and characterization of pH responsive polymeric micelles for the delivery of photosensitizing anticancer drugs J Pharm Sci 89:52 62 Tang X, Gao L, Fan X, Zhou Q 2007 ABA type amphiphilic triblock copolymers containing p ethoxy azobenzene via atom transfer radical polymerization: synthesis, characterization, and properties J Polym Sci Part A: Polym Chem 45:2225 2234 Thurmond KB II, Kowalewski T, Wooley KL 1996 Water soluble knedel like structures: the preparation of shell cross linked small particles J Am Chem Soc 118:7239 7240 Tian Y, Watanabe K, Kong X, Abe J, Iyoda T 2002.

phase /} to phase oc. The values of these quantities and the standard Gibbs energies for the transfer of ions from nitrobenzene or 1,2-dichloroethane into water are listed in Table 3.6. The values of standard Gibbs transfer energies in the water/organic solvent give a quantitative meaning to the terms, hydrophilic and hydrophobic. For hydrophilic ions AG r 'J~^ 0 and the opposite relation is valid for hydrophobic ions. Sometimes the ions with their standard Gibbs transfer energies around zero are called 'semihydrophobic'. Consider a system of two solvents in contact in which a single electrolyte BA is dissolved, consisting of univalent ions. A distribution equilibrium is established between the two solutions. Because, in general, the solvation energies of the anion and cation in the two phases are different so that the ion with a certain charge has a greater tendency to pass into the second phase than the ion of opposite charge, an electrical double layer appears at

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190 the interface (see Section 4.5.3) and a Galvani potential difference is formed between the two phases, called the distribution potential. The value of the distribution potential follows from Eq. (3.2.48). If the activities of the cation and anion in a given phase are set equal to one another and equations of this type calculated once for cations, and then for anions, are added, it follows that

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