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Natansohn A, Rochon P 2002 Photoinduced motions in azo containing polymers Chem Rev 102:4139 4175 Osuji C, Chen JT, Mao G, Ober CK, Thomas EL 2000 Understanding and controlling the morphology of styrene isoprene side group liquid crystalline diblock copolymers Polymer 41:8897 8907 Osuji C, Ferreira P, Mao G, Ober C, Vander J, Thomas EL 2004 Alignment of self assembled hierarchical microstructure in liquid crystalline diblock copolymers using high magnetic elds Macromolecules 37:9903 9908 Osuji C, Zhang Y, Mao G, Ober CK, Thomas EL 1999 Transverse cylindrical micro domain orientation in an LC diblock copolymer under oscillatory shear Macromole cules 32:7703 7706 Paik MY, Krishnan S, You F, Li X, Hexemer A, Ando Y, Kang SH, Fischer DA, Kramer EJ, Ober CK 2007 Surface organization, light driven surface changes, and stability of semi uorinated azobenzene polymers Langmuir 23:5110 5119 Qi B, Yavrian A, Galstian T, Zhao Y 2005.

262 263

(3.2.21)

Liquid crystalline ionomers containing azobenzene mesogens: phase stability, photoinduced birefringence and holographic grating Macromolecules 38:3079 3086 Ravi P, Sin S, Gan L, Gan Y, Tam K, Xia X, Hu X 2005 New water soluble azobenzene containing diblock copolymers: synthesis and aggregation behavior Polymer 46: 137 146 Reiter G, Gastelein G, Hoerner P, Riess G, Blumen A, Sommer J 1999 Nanometer scale surface patterns with long range order created by crystallization of diblock copolymers Phys Rev Lett 83:3844 3847 Rochon P, Batalla E, Natanhson A 1995 Optically induced surface gratings on azoaro matic polymer lms Appl Phys Lett 66:136 138 Rosa CD, Park C, Thomas EL, Lotz B 2003 Microdomain patterns from directional eutectic solidi cation and epitaxy Nature 405:433 437 Saishoji A, Sato D, Shishido A, Ikeda T 2007 Formation of Bragg gratings with large angular multiplicity by means of photoinduced reorientation of azobenzene copolymers Langmuir 23:320 326..

This equation is depicted graphically in Fig. 3.9. Differentiation of the potential E with respect to a yields the following relationship at the point

Drivers Implementation Evaluation Results Environment Benefits Lessons Learned 263 263 263 263 264 264 264

Seki T 2004 Dynamic photoresponsive functions in organized layer systems comprised of azobenzene containing polymers Polym J 36:435 454 Serhatli IE, Serhatli M 1998 Synthesis and characterization of amorphous liquid crystal line poly(vinyl ether) block copolymers Turk J Chem 22:279 287 Sidorenko A, Tokarev I, Minko S, Stamm M 2003 Ordered reactive nanomembranes/ nanotemplates from thin lms of block copolymer supramolecular assembly J Am Chem Soc 125:12211 12216 Suzuki S, Kamata K, Yamauchi H, Iyoda T 2007 Selective doping of lead ions into normally aligned PEO cylindrical nanodomains in amphiphilic block copolymer thin lms Chem Lett 36:978 979 Tang X, Gao L, Fan X, Zhou QF 2007 ABA type amphiphilic triblock copolymers containing p ethoxy azobenzene via atom transfer radical polymerization: synthesis, characterization, and properties J Polym Sci Part A: Polym Chem 45:2225 2234 Thomas EL, Lescanec RL 1994 Phase morphology in block copolymer systems.

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Phil Trans R Soc Lond A 348:149 166 Tian Y, Watanabe K, Kong X, Abe J, Iyoda T 2002 Synthesis, nanostructures, and functionality of amphiphilic liquid crystalline block copolymers with azobenzene moieties Macromolecules 35:3739 3747 Tokita M, Adachi M, Masuyama S, Takazawa F, Watanabe J 2007 Characteristic shear ow orientation in LC block copolymer resulting from compromise between orienta tions of microcylinder and LC mesogen Macromolecules 40:7276 7282 Tokita M, Adachi M, Takazawa F, Watanabe J 2006 Shear ow orientation of cylindrical microdomain in liquid crystalline diblock copolymer and its potentiality as anchoring substrate for nematic mesogens Jpn J Appl Phys 45:9152 9156 Tomikawa N, Lu Z, Itoh T, Imre CT, Adachi M, Tokita M, Watanabe J 2005 Orientation of microphase segregated cylinders in liquid crystalline diblock copolymer by magnetic eld Jpn J Appl Phys 44:L711 L714 Tong X, Cui L, Zhao Y 2004.

At a Glance Organization Drivers Implementation Evaluation Results Environment Benefits Lessons Learned

(3.2.22)

The slope of the tangent to the curve at the inflection point where a = \ is thus inversely proportional to the number of electrons n. The E-oc curves are similar to the titration curves of weak acids or bases (pH-ar). For neutralization curves, the slope dpH/dar characterizes the buffering capacity of the solution; for redox potential curves, the differential dE/da characterizes the redox capacity of the system. If a = ^ for a buffer, then changes in pH produced by changes in a are the smallest possible. If a = \ in a redox system, then the potential changes produced by changes in a are also minimal (the system is 'well poised'). It can be seen from Eq. (3.2.21) that, if the solution contains one of the forms, oxidized or reduced, in zero concentration, then the potential would attain infinite absolute value. These extreme values change to finite values in the presence of a trace of the other form. This always occurs as a result of